1 3
Top Curr Chem (Z) (2018) 376:6
60. Fleischer S, Field RW, Nelson KA (2012) Commensurate two-quantum coherences induced by
time-delayed THz fields. Phys Rev Lett 109:123603. http s://doi.org/10.1103 /Phys RevL ett.109.1236
03
61. Hamm P (2005) Principles of nonlinear optical spectroscopy : a practical approach or : Mukamel
for dummies. University of Zurich. http ://www.mitr .p.lodz .pl/evu/lect ures /Hamm .pdf
62. Tokmakoff A (2014) Time-dependent quantum mechanics and spectroscopy. University of Chicago. http ://tdqm s.uchi cago .edu/
63. Hamm P, Shalit A (2017) Perspective: echoes in 2D-Raman–THz spectroscopy. J Chem Phys
146:130901. http s://doi.org/10.1063 /1.4979 288
64. Tokmakoff A, Lang M, Larsen D et al (1997) Two-dimensional Raman spectroscopy of vibrational
interactions in liquids. Phys Rev Lett 79:2702–2705. http s://doi.org/10.1103 /Phys RevL ett.79.2702
65. Frostig H, Bayer T, Dudovich N et al (2015) Single-beam spectrally controlled two-dimensional
Raman spectroscopy. Nat Photonics 9:339–343. http s://doi.org/10.1038 /npho ton.2015 .64
66. Harde H, Keiding S, Grischkowsky D (1991) THz commensurate echoes: periodic rephasing of
molecular transitions in free-induction decay. Phys Rev Lett 66:1834–1837. http s://doi.org/10.1103
/Phys RevL ett.66.1834
67. Fleischer S, Averbukh IS, Prior Y (2007) Selective alignment of molecular spin isomers. Phys Rev
Lett 99:93002. http s://doi.org/10.1103 /Phys RevL ett.99.0930 02
68. Karras G, Hertz E, Billard F et al (2015) Orientation and alignment echoes. Phys Rev Lett
114:153601. http s://doi.org/10.1103 /Phys RevL ett.114.1536 01
69. Engel GS, Calhoun TR, Read EL et al (2007) Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems. Nature 446:782–786. http s://doi.org/10.1038 /natu re05
678
70. Roberts ST, Loparo JJ, Tokmakoff A (2006) Characterization of spectral diffusion from twodimensional line shapes. J Chem Phys 125:84502. http s://doi.org/10.1063 /1.2232 271
71. Damari R, Kallush S, Fleischer S (2016) Rotational control of asymmetric molecules: dipole- versus polarizability-driven rotational dynamics. Phys Rev Lett 117:103001. http s://doi.org/10.1103 /
Phys RevL ett.117.1030 01
72. Damari R, Rosenberg D, Fleischer S (2017) Coherent radiative decay of molecular rotations: a
comparative study of terahertz-oriented versus optically aligned molecular ensembles. Phys Rev
Lett 119:33002. http s://doi.org/10.1103 /Phys RevL ett.119.0330 02
73. Fecko CJ, Eaves JD, Loparo JJ, Tokmakoff A, Geissler PL (2003) Ultrafast hydrogen-bond dynamics in the infrared spectroscopy of water. Science (80-) 301:1698–1702. http s://doi.org/10.1126 /
scie nce.1087 251
74. Asbury JB, Steinel T, Kwak K et al (2004) Dynamics of water probed with vibrational echo correlation spectroscopy. J Chem Phys 121:12431–12446. http s://doi.org/10.1063 /1.1818 107
75. Hamm P, Savolainen J (2012) Two-dimensional-Raman–terahertz spectroscopy of water: theory. J
Chem Phys 136:94516. http s://doi.org/10.1063 /1.3691 601
76. Hamm P, Savolainen J, Ono J, Tanimura Y (2012) Note: Inverted time-ordering in two-dimensional-Raman–terahertz spectroscopy of water. J Chem Phys 136:236101
77. Teo SM, Ofori-Okai BK, Werley CA, Nelson KA (2015) Invited article: Single-shot THz detection
techniques optimized for multidimensional THz spectroscopy. Rev Sci Instrum 86:51301. http s://
doi.org/10.1063 /1.4921 389
78. Bajaj VS, Mak-Jurkauskas ML, Belenky M et al (2009) Functional and shunt states of bacteriorhodopsin resolved by 250 GHz dynamic nuclear polarization-enhanced solid-state NMR. Proc Natl
Acad Sci USA 106:9244–9249. http s://doi.org/10.1073 /pnas .0900 9081 06
79. Borbat PP, Costa-Filho AJ, Earle KA et al (2001) Electron spin resonance in studies of membranes
and proteins. Science (80-) 291:266–269. http s://doi.org/10.1126 /scie nce.291.5502 .266
80. Koppens FHL, Buizert C, Tielrooij KJ et al (2006) Driven coherent oscillations of a single electron
spin in a quantum dot. Supplementary notes. Nature 442:766–771. http s://doi.org/10.1038 /natu
re05 065
81. Craig GA, Murrie M (2015) 3d single-ion magnets. Chem Soc Rev 44:2135–2147. http s://doi.
org/10.1039 /C4CS 0043 9F
82. Nehrkorn J, Martins BM, Holldack K et al (2013) Zero-field splittings in metHb and metMb
with aquo and fluoro ligands: a FD-FT THz-EPR study. Mol Phys 111:2696–2707. http s://doi.
org/10.1080 /0026 8976 .2013 .8098 06
83. Andersson KK, Schmidt PP, Katterle B et al (2003) Examples of high-frequency EPR studies in
bioinorganic chemistry. J Biol Inorg Chem 8:235–247. http s://doi.org/10.1007 /s007 75-002-0429 -0
319
Reprinted from the journal
Top Curr Chem (Z) (2018) 376:6
60. Fleischer S, Field RW, Nelson KA (2012) Commensurate two-quantum coherences induced by
time-delayed THz fields. Phys Rev Lett 109:123603. http s://doi.org/10.1103 /Phys RevL ett.109.1236
03
61. Hamm P (2005) Principles of nonlinear optical spectroscopy : a practical approach or : Mukamel
for dummies. University of Zurich. http ://www.mitr .p.lodz .pl/evu/lect ures /Hamm .pdf
62. Tokmakoff A (2014) Time-dependent quantum mechanics and spectroscopy. University of Chicago. http ://tdqm s.uchi cago .edu/
63. Hamm P, Shalit A (2017) Perspective: echoes in 2D-Raman–THz spectroscopy. J Chem Phys
146:130901. http s://doi.org/10.1063 /1.4979 288
64. Tokmakoff A, Lang M, Larsen D et al (1997) Two-dimensional Raman spectroscopy of vibrational
interactions in liquids. Phys Rev Lett 79:2702–2705. http s://doi.org/10.1103 /Phys RevL ett.79.2702
65. Frostig H, Bayer T, Dudovich N et al (2015) Single-beam spectrally controlled two-dimensional
Raman spectroscopy. Nat Photonics 9:339–343. http s://doi.org/10.1038 /npho ton.2015 .64
66. Harde H, Keiding S, Grischkowsky D (1991) THz commensurate echoes: periodic rephasing of
molecular transitions in free-induction decay. Phys Rev Lett 66:1834–1837. http s://doi.org/10.1103
/Phys RevL ett.66.1834
67. Fleischer S, Averbukh IS, Prior Y (2007) Selective alignment of molecular spin isomers. Phys Rev
Lett 99:93002. http s://doi.org/10.1103 /Phys RevL ett.99.0930 02
68. Karras G, Hertz E, Billard F et al (2015) Orientation and alignment echoes. Phys Rev Lett
114:153601. http s://doi.org/10.1103 /Phys RevL ett.114.1536 01
69. Engel GS, Calhoun TR, Read EL et al (2007) Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems. Nature 446:782–786. http s://doi.org/10.1038 /natu re05
678
70. Roberts ST, Loparo JJ, Tokmakoff A (2006) Characterization of spectral diffusion from twodimensional line shapes. J Chem Phys 125:84502. http s://doi.org/10.1063 /1.2232 271
71. Damari R, Kallush S, Fleischer S (2016) Rotational control of asymmetric molecules: dipole- versus polarizability-driven rotational dynamics. Phys Rev Lett 117:103001. http s://doi.org/10.1103 /
Phys RevL ett.117.1030 01
72. Damari R, Rosenberg D, Fleischer S (2017) Coherent radiative decay of molecular rotations: a
comparative study of terahertz-oriented versus optically aligned molecular ensembles. Phys Rev
Lett 119:33002. http s://doi.org/10.1103 /Phys RevL ett.119.0330 02
73. Fecko CJ, Eaves JD, Loparo JJ, Tokmakoff A, Geissler PL (2003) Ultrafast hydrogen-bond dynamics in the infrared spectroscopy of water. Science (80-) 301:1698–1702. http s://doi.org/10.1126 /
scie nce.1087 251
74. Asbury JB, Steinel T, Kwak K et al (2004) Dynamics of water probed with vibrational echo correlation spectroscopy. J Chem Phys 121:12431–12446. http s://doi.org/10.1063 /1.1818 107
75. Hamm P, Savolainen J (2012) Two-dimensional-Raman–terahertz spectroscopy of water: theory. J
Chem Phys 136:94516. http s://doi.org/10.1063 /1.3691 601
76. Hamm P, Savolainen J, Ono J, Tanimura Y (2012) Note: Inverted time-ordering in two-dimensional-Raman–terahertz spectroscopy of water. J Chem Phys 136:236101
77. Teo SM, Ofori-Okai BK, Werley CA, Nelson KA (2015) Invited article: Single-shot THz detection
techniques optimized for multidimensional THz spectroscopy. Rev Sci Instrum 86:51301. http s://
doi.org/10.1063 /1.4921 389
78. Bajaj VS, Mak-Jurkauskas ML, Belenky M et al (2009) Functional and shunt states of bacteriorhodopsin resolved by 250 GHz dynamic nuclear polarization-enhanced solid-state NMR. Proc Natl
Acad Sci USA 106:9244–9249. http s://doi.org/10.1073 /pnas .0900 9081 06
79. Borbat PP, Costa-Filho AJ, Earle KA et al (2001) Electron spin resonance in studies of membranes
and proteins. Science (80-) 291:266–269. http s://doi.org/10.1126 /scie nce.291.5502 .266
80. Koppens FHL, Buizert C, Tielrooij KJ et al (2006) Driven coherent oscillations of a single electron
spin in a quantum dot. Supplementary notes. Nature 442:766–771. http s://doi.org/10.1038 /natu
re05 065
81. Craig GA, Murrie M (2015) 3d single-ion magnets. Chem Soc Rev 44:2135–2147. http s://doi.
org/10.1039 /C4CS 0043 9F
82. Nehrkorn J, Martins BM, Holldack K et al (2013) Zero-field splittings in metHb and metMb
with aquo and fluoro ligands: a FD-FT THz-EPR study. Mol Phys 111:2696–2707. http s://doi.
org/10.1080 /0026 8976 .2013 .8098 06
83. Andersson KK, Schmidt PP, Katterle B et al (2003) Examples of high-frequency EPR studies in
bioinorganic chemistry. J Biol Inorg Chem 8:235–247. http s://doi.org/10.1007 /s007 75-002-0429 -0
319
Reprinted from the journal