1 3
Top Curr Chem (Z) (2018) 376:6
16. Blanchard F, Razzari L, Bandulet HC et al (2007) Generation of 1.5 µJ single-cycle terahertz
pulses by optical rectification from a large aperture ZnTe crystal. Opt Express 15:13212. http s://
doi.org/10.1364 /OE.15.0132 12
17. Ferguson B, Zhang X-C (2002) Materials for terahertz science and technology. Nat Mater 1:26–33.
http s://doi.org/10.1038 /nmat 708
18. Schmuttenmaer CA (2004) Exploring dynamics in the far-infrared with terahertz spectroscopy.
Chem Rev 104:1759–1779. http s://doi.org/10.1021 /cr02 0685 g
19. Tonouchi M (2007) Cutting-edge terahertz technology. Nat Photonics 1:97–105. http s://doi.
org/10.1038 /npho ton.2007 .3
20. Yeh KL, Hoffmann MC, Hebling J, Nelson KA (2007) Generation of 10 μJ ultrashort terahertz
pulses by optical rectification. Appl Phys Lett 90:171121. http s://doi.org/10.1063 /1.2734 374
21. Hirori H, Doi A, Blanchard F, Tanaka K (2011) Single-cycle terahertz pulses with amplitudes
exceeding 1 MV/cm generated by optical rectification in LiNbO 3 . Appl Phys Lett 98:91106. http s://
doi.org/10.1063 /1.3560 062
22. Shalaby M, Hauri CP (2015) Demonstration of a low-frequency three-dimensional terahertz bullet
with extreme brightness. Nat Commun 6:5976. http s://doi.org/10.1038 /ncom ms69 76
23. Vicario C, Ruchert C, Hauri CP (2015) High field broadband THz generation in organic materials.
J Mod Opt 62:1480–1485. http s://doi.org/10.1080 /0950 0340 .2013 .8002 42
24. Lee S-H, Jazbinsek M, Hauri CP, Kwon O-P (2016) Recent progress in acentric core structures for
highly efficient nonlinear optical crystals and their supramolecular interactions and terahertz applications. CrystEngComm 18:7180–7203. http s://doi.org/10.1039 /C6CE 0070 7D
25. Kampfrath T, Tanaka K, Nelson KA (2013) Resonant and nonresonant control over matter and
light by intense terahertz transients. Nat Photonics 7:680–690. http s://doi.org/10.1038 /npho
ton.2013 .184
26. Hwang HY, Fleischer S, Brandt NC et al (2015) A review of non-linear terahertz spectroscopy with
ultrashort tabletop-laser pulses. J Mod Opt 62:1447–1479. http s://doi.org/10.1080 /0950 0340 .2014
.9182 00
27. Woerner M, Kuehn W, Bowlan P et al (2013) Ultrafast two-dimensional terahertz spectroscopy
of elementary excitations in solids. New J Phys 15:25039. http s://doi.org/10.1088 /1367 -2630
/15/2/0250 39
28. Kuehn W, Reimann K, Woerner M et al (2011) Strong correlation of electronic and lattice excitations in GaAs/AlGaAs semiconductor quantum wells revealed by two-dimensional terahertz spectroscopy. Phys Rev Lett 107:67401. http s://doi.org/10.1103 /Phys RevL ett.107.0674 01
29. Somma C, Reimann K, Flytzanis C et al (2014) High-field terahertz bulk photovoltaic effect in
lithium niobate. Phys Rev Lett 112:146602. http s://doi.org/10.1103 /Phys RevL ett.112.1466 02
30. Maag T, Bayer A, Baierl S et al (2015) Coherent cyclotron motion beyond Kohn’s theorem. Nat
Phys 11:1–6. http s://doi.org/10.1038 /NPHY S355 9
31. Lu J, Zhang Y, Hwang HY et al (2016) Nonlinear two-dimensional terahertz photon echo and
rotational spectroscopy in the gas phase. Proc Natl Acad Sci USA 113:11800–11805. http s://doi.
org/10.1073 /pnas .1609 5581 13
32. Lu J, Zhang Y, Hwang HY et al (2016) Two-dimensional terahertz photon echo and rotational
spectroscopy in the gas phase. In: International conference on ultrafast phenomena. OSA Technical Digest (online), Optical Society of America, Paper UTu1A.6. http s://doi.org/10.1364 /UP.2016
.UTu1 A.6
33. Somma C, Folpini G, Reimann K et al (2016) Two-phonon quantum coherences in indium antimonide studied by nonlinear two-dimensional terahertz spectroscopy. Phys Rev Lett 116:1–6. http s://
doi.org/10.1103 /Phys RevL ett.116.1774 01
34. Somma C, Folpini G, Reimann K et al (2016) Phase-resolved two-dimensional terahertz spectroscopy including off-resonant interactions beyond the χ
(3) limit. J Chem Phys 144:184202. http s://
doi.org/10.1063 /1.4948 639
35. Lu J, Li X, Hwang HY et al (2016) 2D nonlinear terahertz magnetic resonance spectroscopy of
magnons in a canted antiferromagnet. In: International conference on ultrafast phenomena. OSA
Technical Digest (online), Optical Society of America, Paper UTh3A.2. http s://doi.org/10.1364 /
UP.2016 .UTh3 A.2
36. Lu J, Li X, Hwang HY et al (2017) Coherent two-dimensional terahertz magnetic resonance spectroscopy of collective spin waves. Phys Rev Lett 118:207204. http s://doi.org/10.1103 /Phys RevL
ett.118.2072 04
317
Reprinted from the journal
Top Curr Chem (Z) (2018) 376:6
16. Blanchard F, Razzari L, Bandulet HC et al (2007) Generation of 1.5 µJ single-cycle terahertz
pulses by optical rectification from a large aperture ZnTe crystal. Opt Express 15:13212. http s://
doi.org/10.1364 /OE.15.0132 12
17. Ferguson B, Zhang X-C (2002) Materials for terahertz science and technology. Nat Mater 1:26–33.
http s://doi.org/10.1038 /nmat 708
18. Schmuttenmaer CA (2004) Exploring dynamics in the far-infrared with terahertz spectroscopy.
Chem Rev 104:1759–1779. http s://doi.org/10.1021 /cr02 0685 g
19. Tonouchi M (2007) Cutting-edge terahertz technology. Nat Photonics 1:97–105. http s://doi.
org/10.1038 /npho ton.2007 .3
20. Yeh KL, Hoffmann MC, Hebling J, Nelson KA (2007) Generation of 10 μJ ultrashort terahertz
pulses by optical rectification. Appl Phys Lett 90:171121. http s://doi.org/10.1063 /1.2734 374
21. Hirori H, Doi A, Blanchard F, Tanaka K (2011) Single-cycle terahertz pulses with amplitudes
exceeding 1 MV/cm generated by optical rectification in LiNbO 3 . Appl Phys Lett 98:91106. http s://
doi.org/10.1063 /1.3560 062
22. Shalaby M, Hauri CP (2015) Demonstration of a low-frequency three-dimensional terahertz bullet
with extreme brightness. Nat Commun 6:5976. http s://doi.org/10.1038 /ncom ms69 76
23. Vicario C, Ruchert C, Hauri CP (2015) High field broadband THz generation in organic materials.
J Mod Opt 62:1480–1485. http s://doi.org/10.1080 /0950 0340 .2013 .8002 42
24. Lee S-H, Jazbinsek M, Hauri CP, Kwon O-P (2016) Recent progress in acentric core structures for
highly efficient nonlinear optical crystals and their supramolecular interactions and terahertz applications. CrystEngComm 18:7180–7203. http s://doi.org/10.1039 /C6CE 0070 7D
25. Kampfrath T, Tanaka K, Nelson KA (2013) Resonant and nonresonant control over matter and
light by intense terahertz transients. Nat Photonics 7:680–690. http s://doi.org/10.1038 /npho
ton.2013 .184
26. Hwang HY, Fleischer S, Brandt NC et al (2015) A review of non-linear terahertz spectroscopy with
ultrashort tabletop-laser pulses. J Mod Opt 62:1447–1479. http s://doi.org/10.1080 /0950 0340 .2014
.9182 00
27. Woerner M, Kuehn W, Bowlan P et al (2013) Ultrafast two-dimensional terahertz spectroscopy
of elementary excitations in solids. New J Phys 15:25039. http s://doi.org/10.1088 /1367 -2630
/15/2/0250 39
28. Kuehn W, Reimann K, Woerner M et al (2011) Strong correlation of electronic and lattice excitations in GaAs/AlGaAs semiconductor quantum wells revealed by two-dimensional terahertz spectroscopy. Phys Rev Lett 107:67401. http s://doi.org/10.1103 /Phys RevL ett.107.0674 01
29. Somma C, Reimann K, Flytzanis C et al (2014) High-field terahertz bulk photovoltaic effect in
lithium niobate. Phys Rev Lett 112:146602. http s://doi.org/10.1103 /Phys RevL ett.112.1466 02
30. Maag T, Bayer A, Baierl S et al (2015) Coherent cyclotron motion beyond Kohn’s theorem. Nat
Phys 11:1–6. http s://doi.org/10.1038 /NPHY S355 9
31. Lu J, Zhang Y, Hwang HY et al (2016) Nonlinear two-dimensional terahertz photon echo and
rotational spectroscopy in the gas phase. Proc Natl Acad Sci USA 113:11800–11805. http s://doi.
org/10.1073 /pnas .1609 5581 13
32. Lu J, Zhang Y, Hwang HY et al (2016) Two-dimensional terahertz photon echo and rotational
spectroscopy in the gas phase. In: International conference on ultrafast phenomena. OSA Technical Digest (online), Optical Society of America, Paper UTu1A.6. http s://doi.org/10.1364 /UP.2016
.UTu1 A.6
33. Somma C, Folpini G, Reimann K et al (2016) Two-phonon quantum coherences in indium antimonide studied by nonlinear two-dimensional terahertz spectroscopy. Phys Rev Lett 116:1–6. http s://
doi.org/10.1103 /Phys RevL ett.116.1774 01
34. Somma C, Folpini G, Reimann K et al (2016) Phase-resolved two-dimensional terahertz spectroscopy including off-resonant interactions beyond the χ
(3) limit. J Chem Phys 144:184202. http s://
doi.org/10.1063 /1.4948 639
35. Lu J, Li X, Hwang HY et al (2016) 2D nonlinear terahertz magnetic resonance spectroscopy of
magnons in a canted antiferromagnet. In: International conference on ultrafast phenomena. OSA
Technical Digest (online), Optical Society of America, Paper UTh3A.2. http s://doi.org/10.1364 /
UP.2016 .UTh3 A.2
36. Lu J, Li X, Hwang HY et al (2017) Coherent two-dimensional terahertz magnetic resonance spectroscopy of collective spin waves. Phys Rev Lett 118:207204. http s://doi.org/10.1103 /Phys RevL
ett.118.2072 04
317
Reprinted from the journal