1 3
Topics in Current Chemistry (2018) 376:28
57. Buckup T, Kraack JP, Marek MS, Motzkus M (2013) Vibronic coupling in excited electronic states
investigated with resonant 2D Raman spectroscopy. In: XVIIIth international conference on ultrafast phenomena. Vol 41 p 05018. https ://doi.org/10.1051/epjco nf/20134 10501 8
58. Bredenbeck J, Helbing J, Behrendt R, Renner C, Moroder L, Wachtveitl J, Hamm P (2003) Transient 2D-IR spectroscopy: snapshots of the nonequilibrium ensemble during the picosecond
conformational transition of a small peptide. J Phys Chem B 107(33):8654–8660. https ://doi.
org/10.1021/jp034 552q
59. Kolano C, Helbing J, Kozinski M, Sander W, Hamm P (2006) Watching hydrogen-bond dynamics in a beta-turn by transient two-dimensional infrared spectroscopy. Nature 444(7118):469–472.
https ://doi.org/10.1038/natur e0535 2
60. Chung HS, Ganim Z, Jones KC, Tokmakoff A (2007) Transient 2D IR spectroscopy of ubiquitin unfolding dynamics. Proc Natl Acad Sci 104(36):14237–14242. https ://doi.org/10.1073/
pnas.07009 59104
61. Goodno GD, Dadusc G, Miller RJD (1998) Ultrafast heterodyne-detected transient-grating
spectroscopy using diffractive optics. J Opt Soc Am B Opt Phys 15(6):1791–1794. https ://doi.
org/10.1364/josab .15.00179 1
62. Lepetit L, Cheriaux G, Joffre M (1995) Linear techniques of phase measurement by femtosecond
spectral interferometry for applications in spectroscopy. J Opt Soc Am B Opt Phys 12(12):2467–
2474. https ://doi.org/10.1364/josab .12.00246 7
63. Tokmakoff A, Lang MJ, Larsen DS, Fleming GR (1997) Intrinsic optical heterodyne detection
of a two-dimensional fifth order Raman response. Chem Phys Lett 272(1–2):48–54. https ://doi.
org/10.1016/s0009 -2614(97)00479 -x
64. Krebs N, Pugliesi I, Hauer J, Riedle E (2013) Two-dimensional Fourier transform spectroscopy
in the ultraviolet with sub-20 fs pump pulses and 250–720 nm supercontinuum probe. New J Phys
15:17. https ://doi.org/10.1088/1367-2630/15/8/08501 6
65. Dadusc G, Ogilvie JP, Schulenberg P, Marvet U, Miller RJD (2001) Diffractive optics-based heterodyne-detected four-wave mixing signals of protein motion: from “protein quakes” to ligand escape
for myoglobin. Proc Natl Acad Sci USA 98(11):6110–6115. https ://doi.org/10.1073/pnas.10113
0298
66. Kubarych KJ, Milne CJ, Lin S, Astinov V, Miller RJD (2002) Diffractive optics-based six-wave
mixing: heterodyne detection of the full chi(5) tensor of liquid CS2. J Chem Phys 116(5):2016–
2042. https ://doi.org/10.1063/1.14299 61
67. Cowan ML, Ogilvie JP, Miller RJD (2004) Two-dimensional spectroscopy using diffractive optics
based phased-locked photon echoes. Chem Phys Lett 386(1–3):184–189. https ://doi.org/10.1016/j.
cplet t.2004.01.027
68. Brixner T, Mancal T, Stiopkin IV, Fleming GR (2004) Phase-stabilized two-dimensional electronic
spectroscopy. J Chem Phys 121(9):4221–4236. https ://doi.org/10.1063/1.17761 12
69. Brixner T, Stiopkin IV, Fleming GR (2004) Tunable two-dimensional femtosecond spectroscopy.
Opt Lett 29(8):884–886. https ://doi.org/10.1364/ol.29.00088 4
70. Shim SH, Strasfeld DB, Zanni MT (2006) Generation and characterization of phase and amplitude
shaped femtosecond mid-IR pulses. Opt Express 14(26):13120–13130. https ://doi.org/10.1364/
oe.14.01312 0
71. Shim SH, Strasfeld DB, Ling YL, Zanni MT (2007) Automated 2D IR spectroscopy using a midIR pulse shaper and application of this technology to the human islet amyloid polypeptide. Proc
Natl Acad Sci USA 104(36):14197–14202. https ://doi.org/10.1073/pnas.07008 04104
72. Shim SH, Zanni MT (2009) How to turn your pump-probe instrument into a multidimensional
spectrometer: 2D IR and Vis spectroscopies via pulse shaping. Phys Chem Chem Phys 11(5):748–
761. https ://doi.org/10.1039/b8138 17f
73. Gundogdu K, Stone KW, Turner DB, Nelson KA (2007) Multidimensional coherent spectroscopy
made easy. Chem Phys 341(1–3):89–94. https ://doi.org/10.1016/j.chemp hys.2007.06.027
74. Hornung T, Vaughan JC, Feurer T, Nelson KA (2004) Degenerate four-wave mixing spectroscopy
based on two-dimensional femtosecond pulse shaping. Opt Lett 29(17):2052–2054. https ://doi.
org/10.1364/ol.29.00205 2
75. Vaughan JC, Hornung T, Stone KW, Nelson KA (2007) Coherently controlled ultrafast four-wave
mixing spectroscopy. J Phys Chem A 111(23):4873–4883. https ://doi.org/10.1021/jp066 2911
76. Shim S-H, Strasfeld DB, Ling YL, Zanni MT (2007) Automated 2D IR spectroscopy using a midIR pulse shaper and application of this technology to the human islet amyloid polypeptide. Proc
Natl Acad Sci USA 104(36):14197–14202. https ://doi.org/10.1073/pnas.07008 04104
21
Reprinted from the journal
Topics in Current Chemistry (2018) 376:28
57. Buckup T, Kraack JP, Marek MS, Motzkus M (2013) Vibronic coupling in excited electronic states
investigated with resonant 2D Raman spectroscopy. In: XVIIIth international conference on ultrafast phenomena. Vol 41 p 05018. https ://doi.org/10.1051/epjco nf/20134 10501 8
58. Bredenbeck J, Helbing J, Behrendt R, Renner C, Moroder L, Wachtveitl J, Hamm P (2003) Transient 2D-IR spectroscopy: snapshots of the nonequilibrium ensemble during the picosecond
conformational transition of a small peptide. J Phys Chem B 107(33):8654–8660. https ://doi.
org/10.1021/jp034 552q
59. Kolano C, Helbing J, Kozinski M, Sander W, Hamm P (2006) Watching hydrogen-bond dynamics in a beta-turn by transient two-dimensional infrared spectroscopy. Nature 444(7118):469–472.
https ://doi.org/10.1038/natur e0535 2
60. Chung HS, Ganim Z, Jones KC, Tokmakoff A (2007) Transient 2D IR spectroscopy of ubiquitin unfolding dynamics. Proc Natl Acad Sci 104(36):14237–14242. https ://doi.org/10.1073/
pnas.07009 59104
61. Goodno GD, Dadusc G, Miller RJD (1998) Ultrafast heterodyne-detected transient-grating
spectroscopy using diffractive optics. J Opt Soc Am B Opt Phys 15(6):1791–1794. https ://doi.
org/10.1364/josab .15.00179 1
62. Lepetit L, Cheriaux G, Joffre M (1995) Linear techniques of phase measurement by femtosecond
spectral interferometry for applications in spectroscopy. J Opt Soc Am B Opt Phys 12(12):2467–
2474. https ://doi.org/10.1364/josab .12.00246 7
63. Tokmakoff A, Lang MJ, Larsen DS, Fleming GR (1997) Intrinsic optical heterodyne detection
of a two-dimensional fifth order Raman response. Chem Phys Lett 272(1–2):48–54. https ://doi.
org/10.1016/s0009 -2614(97)00479 -x
64. Krebs N, Pugliesi I, Hauer J, Riedle E (2013) Two-dimensional Fourier transform spectroscopy
in the ultraviolet with sub-20 fs pump pulses and 250–720 nm supercontinuum probe. New J Phys
15:17. https ://doi.org/10.1088/1367-2630/15/8/08501 6
65. Dadusc G, Ogilvie JP, Schulenberg P, Marvet U, Miller RJD (2001) Diffractive optics-based heterodyne-detected four-wave mixing signals of protein motion: from “protein quakes” to ligand escape
for myoglobin. Proc Natl Acad Sci USA 98(11):6110–6115. https ://doi.org/10.1073/pnas.10113
0298
66. Kubarych KJ, Milne CJ, Lin S, Astinov V, Miller RJD (2002) Diffractive optics-based six-wave
mixing: heterodyne detection of the full chi(5) tensor of liquid CS2. J Chem Phys 116(5):2016–
2042. https ://doi.org/10.1063/1.14299 61
67. Cowan ML, Ogilvie JP, Miller RJD (2004) Two-dimensional spectroscopy using diffractive optics
based phased-locked photon echoes. Chem Phys Lett 386(1–3):184–189. https ://doi.org/10.1016/j.
cplet t.2004.01.027
68. Brixner T, Mancal T, Stiopkin IV, Fleming GR (2004) Phase-stabilized two-dimensional electronic
spectroscopy. J Chem Phys 121(9):4221–4236. https ://doi.org/10.1063/1.17761 12
69. Brixner T, Stiopkin IV, Fleming GR (2004) Tunable two-dimensional femtosecond spectroscopy.
Opt Lett 29(8):884–886. https ://doi.org/10.1364/ol.29.00088 4
70. Shim SH, Strasfeld DB, Zanni MT (2006) Generation and characterization of phase and amplitude
shaped femtosecond mid-IR pulses. Opt Express 14(26):13120–13130. https ://doi.org/10.1364/
oe.14.01312 0
71. Shim SH, Strasfeld DB, Ling YL, Zanni MT (2007) Automated 2D IR spectroscopy using a midIR pulse shaper and application of this technology to the human islet amyloid polypeptide. Proc
Natl Acad Sci USA 104(36):14197–14202. https ://doi.org/10.1073/pnas.07008 04104
72. Shim SH, Zanni MT (2009) How to turn your pump-probe instrument into a multidimensional
spectrometer: 2D IR and Vis spectroscopies via pulse shaping. Phys Chem Chem Phys 11(5):748–
761. https ://doi.org/10.1039/b8138 17f
73. Gundogdu K, Stone KW, Turner DB, Nelson KA (2007) Multidimensional coherent spectroscopy
made easy. Chem Phys 341(1–3):89–94. https ://doi.org/10.1016/j.chemp hys.2007.06.027
74. Hornung T, Vaughan JC, Feurer T, Nelson KA (2004) Degenerate four-wave mixing spectroscopy
based on two-dimensional femtosecond pulse shaping. Opt Lett 29(17):2052–2054. https ://doi.
org/10.1364/ol.29.00205 2
75. Vaughan JC, Hornung T, Stone KW, Nelson KA (2007) Coherently controlled ultrafast four-wave
mixing spectroscopy. J Phys Chem A 111(23):4873–4883. https ://doi.org/10.1021/jp066 2911
76. Shim S-H, Strasfeld DB, Ling YL, Zanni MT (2007) Automated 2D IR spectroscopy using a midIR pulse shaper and application of this technology to the human islet amyloid polypeptide. Proc
Natl Acad Sci USA 104(36):14197–14202. https ://doi.org/10.1073/pnas.07008 04104
21
Reprinted from the journal