4.5 Results and Discussion
137
Fig. 4.14 Construction of the two-layered approach for vibrational up-pumping for α-FOX-7.
(Top) The phonon density of states (blue) is shown, along with the first overtone density of states
(green). (Bottom) Recasting the overtone populations onto the phonon density of states in the region
max < ω < 2 max (highlighted by red box)
4.5.3.4 Temperature Dependent Up-Pumping
It follows from Sect. 4.5.3.2 that simple counting of the number of up-pumping
pathways is not the best indicator to describe the relative sensitivities of the molecular
137
Fig. 4.14 Construction of the two-layered approach for vibrational up-pumping for α-FOX-7.
(Top) The phonon density of states (blue) is shown, along with the first overtone density of states
(green). (Bottom) Recasting the overtone populations onto the phonon density of states in the region
max < ω < 2 max (highlighted by red box)
4.5.3.4 Temperature Dependent Up-Pumping
It follows from Sect. 4.5.3.2 that simple counting of the number of up-pumping
pathways is not the best indicator to describe the relative sensitivities of the molecular