References
1. S. Kielich, Molekularna Optyka Nieliniowa (Nonlinear Molecular Optics) (Naukowe,
Warszawa-Poznan, 1977)
2. H.J. Achtermann, G. Magnus, T.K. Bose, Refractivity virial coefficients of gaseous CH 4 ,
C 2 H 4 , C 2 H 6 , CO 2 , SF 6 , H 2 , N 2 , He and Ar. J. Chem. Phys. 94(8), 5669–5684 (1991)
3. U. Hohm, K. Kerl, A Michelson twin interferometer for precise measurements of refractive
index of gases between 100 K and 1300 K. Meas. Sci. Technol. 1(4), 329–336 (1990)
4. U. Hohm, K. Kerl, Interferometric measurements of dipole polarizability α; of molecules
between 300 K and 1100 K. II. A new method measuring the dispersion of the polarizability
and its application to Ar, H 2 , and O 2 . Mol. Phys. 69(5), 819–831 (1990)
5. K. Kerl, U. Hohm, H. Varchmin, Polarizability α(ω, T, ρ) of small molecules in the gas
phase. Ber. Bunsenges. Phys. Chem. 96(5), 728–733 (1992)
6. U. Hohm, Frequency-dependence of second refractivity virial coefficients of small molecules
between 325 nm and 633 nm. Mol. Phys. 81(1), 157–168 (1994)
7. M. Monan, J.-L. Bribes, R. Gaufres, Measurement of weak depolarization ratios of the
Rayleigh scattering of gases using Raman spectroscopy. J. Raman Spectroscopy 12(2), 190–
193 (1982)
8. X. Song, J. Jonas, T.W. Zerda, Total intensity measurements of depolarized Rayleigh
scattering from linear molecules. J. Phys. Chem. 93(19), 6887–6890 (1989)
Table 4.1 (continued)
R, Å
Config.
α xx
α yy
α zz
Config.
α xx
α yy
α zz
10
58.96
58.96
44.37
58.93
43.95
59.71
3.5
5
43.99
54.04
62.81
11
63.03
44.32
52.01
4
44.81
55.44
61.71
64.44
45.06
51.06
4.5
45.40
56.47
60.87
65.45
45.57
50.21
5
45.81
57.18
60.05
66.16
45.92
49.48
5.5
46.10
57.67
59.30
66.67
46.16
48.91
6
46.30
58.01
58.68
67.04
46.34
48.48
7
46.55
58.45
57.86
67.54
46.58
47.94
8
46.70
58.69
57.40
67.84
46.71
47.63
9
46.79
58.84
57.13
68.02
46.80
47.45
10
46.85
58.94
56.96
68.14
46.85
47.34
3.5
6
55.37
52.59
51.38
12
62.25
41.04
57.07
4
56.34
53.58
50.81
63.95
41.94
55.19
4.5
57.04
54.28
50.11
65.13
42.55
53.81
5
57.54
54.76
49.44
66.11
43.11
52.94
5.5
57.90
55.11
48.89
66.71
43.42
52.26
6
58.17
55.36
48.48
67.12
43.61
51.75
7
58.52
55.68
47.94
67.67
43.85
51.13
8
58.74
55.88
47.63
67.99
43.99
50.79
9
58.87
56.00
47.45
68.18
44.08
50.59
10
58.96
56.07
47.34
68.31
44.13
50.46
76
4 Interaction-induced Polarizability
1. S. Kielich, Molekularna Optyka Nieliniowa (Nonlinear Molecular Optics) (Naukowe,
Warszawa-Poznan, 1977)
2. H.J. Achtermann, G. Magnus, T.K. Bose, Refractivity virial coefficients of gaseous CH 4 ,
C 2 H 4 , C 2 H 6 , CO 2 , SF 6 , H 2 , N 2 , He and Ar. J. Chem. Phys. 94(8), 5669–5684 (1991)
3. U. Hohm, K. Kerl, A Michelson twin interferometer for precise measurements of refractive
index of gases between 100 K and 1300 K. Meas. Sci. Technol. 1(4), 329–336 (1990)
4. U. Hohm, K. Kerl, Interferometric measurements of dipole polarizability α; of molecules
between 300 K and 1100 K. II. A new method measuring the dispersion of the polarizability
and its application to Ar, H 2 , and O 2 . Mol. Phys. 69(5), 819–831 (1990)
5. K. Kerl, U. Hohm, H. Varchmin, Polarizability α(ω, T, ρ) of small molecules in the gas
phase. Ber. Bunsenges. Phys. Chem. 96(5), 728–733 (1992)
6. U. Hohm, Frequency-dependence of second refractivity virial coefficients of small molecules
between 325 nm and 633 nm. Mol. Phys. 81(1), 157–168 (1994)
7. M. Monan, J.-L. Bribes, R. Gaufres, Measurement of weak depolarization ratios of the
Rayleigh scattering of gases using Raman spectroscopy. J. Raman Spectroscopy 12(2), 190–
193 (1982)
8. X. Song, J. Jonas, T.W. Zerda, Total intensity measurements of depolarized Rayleigh
scattering from linear molecules. J. Phys. Chem. 93(19), 6887–6890 (1989)
Table 4.1 (continued)
R, Å
Config.
α xx
α yy
α zz
Config.
α xx
α yy
α zz
10
58.96
58.96
44.37
58.93
43.95
59.71
3.5
5
43.99
54.04
62.81
11
63.03
44.32
52.01
4
44.81
55.44
61.71
64.44
45.06
51.06
4.5
45.40
56.47
60.87
65.45
45.57
50.21
5
45.81
57.18
60.05
66.16
45.92
49.48
5.5
46.10
57.67
59.30
66.67
46.16
48.91
6
46.30
58.01
58.68
67.04
46.34
48.48
7
46.55
58.45
57.86
67.54
46.58
47.94
8
46.70
58.69
57.40
67.84
46.71
47.63
9
46.79
58.84
57.13
68.02
46.80
47.45
10
46.85
58.94
56.96
68.14
46.85
47.34
3.5
6
55.37
52.59
51.38
12
62.25
41.04
57.07
4
56.34
53.58
50.81
63.95
41.94
55.19
4.5
57.04
54.28
50.11
65.13
42.55
53.81
5
57.54
54.76
49.44
66.11
43.11
52.94
5.5
57.90
55.11
48.89
66.71
43.42
52.26
6
58.17
55.36
48.48
67.12
43.61
51.75
7
58.52
55.68
47.94
67.67
43.85
51.13
8
58.74
55.88
47.63
67.99
43.99
50.79
9
58.87
56.00
47.45
68.18
44.08
50.59
10
58.96
56.07
47.34
68.31
44.13
50.46
76
4 Interaction-induced Polarizability