Contents
1
Molecular Movies from Molecular Frame Photoelectron Angular
Distribution (MF-PAD) Measurements . . . . . . . . . . . . . . . .
1
Arnaud Rouzée, Ymkje Huismans, Freek Kelkensberg, Aneta
Smolkowska, Julia H. Jungmann, Arjan Gijsbertsen, Wing Kiu Siu,
Georg Gademann, Axel Hundertmark, Per Johnsson, and Marc J.J.
Vrakking
1.1 Introduction . . . . . . . . . . . . . . . . . . . . . . . . . . . .
1
1.2 Molecular Movies Using XUV/X-Ray Photoionization . . . . . .
5
1.3 Molecular Movies Using Strong Field Mid-Infrared Ionization . .
14
1.4 Outlook . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .
20
References . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .
22
2
XUV Lasers for Ultrafast Electronic Control in H 2 . . . . . . . . .
25
Alicia Palacios, Paula Rivière, Alberto González-Castrillo, and
Fernando Martín
2.1 Introduction . . . . . . . . . . . . . . . . . . . . . . . . . . . .
26
2.2 Experimental Set-Ups . . . . . . . . . . . . . . . . . . . . . . .
27
2.3 Theoretical Approach and Implementation . . . . . . . . . . . .
28
2.3.1 Time-Dependent Spectral Method . . . . . . . . . . . . .
29
2.4 Time-Resolved Imaging of H 2 Autoionization . . . . . . . . . .
32
2.5 Control and Non-linear Effects in Multiphoton Single Ionization
37
2.5.1 Control of Single Ionization Channels by Means of VUV
Pulses . . . . . . . . . . . . . . . . . . . . . . . . . . .
37
2.5.2 Non-linear Effects in (1 + 1)-REMPI . . . . . . . . . . .
39
2.5.3 Probing Nuclear Wave Packets in Molecular Excited
States . . . . . . . . . . . . . . . . . . . . . . . . . . . .
43
2.6 Future Perspectives . . . . . . . . . . . . . . . . . . . . . . . .
45
References . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .
46
ix
1
Molecular Movies from Molecular Frame Photoelectron Angular
Distribution (MF-PAD) Measurements . . . . . . . . . . . . . . . .
1
Arnaud Rouzée, Ymkje Huismans, Freek Kelkensberg, Aneta
Smolkowska, Julia H. Jungmann, Arjan Gijsbertsen, Wing Kiu Siu,
Georg Gademann, Axel Hundertmark, Per Johnsson, and Marc J.J.
Vrakking
1.1 Introduction . . . . . . . . . . . . . . . . . . . . . . . . . . . .
1
1.2 Molecular Movies Using XUV/X-Ray Photoionization . . . . . .
5
1.3 Molecular Movies Using Strong Field Mid-Infrared Ionization . .
14
1.4 Outlook . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .
20
References . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .
22
2
XUV Lasers for Ultrafast Electronic Control in H 2 . . . . . . . . .
25
Alicia Palacios, Paula Rivière, Alberto González-Castrillo, and
Fernando Martín
2.1 Introduction . . . . . . . . . . . . . . . . . . . . . . . . . . . .
26
2.2 Experimental Set-Ups . . . . . . . . . . . . . . . . . . . . . . .
27
2.3 Theoretical Approach and Implementation . . . . . . . . . . . .
28
2.3.1 Time-Dependent Spectral Method . . . . . . . . . . . . .
29
2.4 Time-Resolved Imaging of H 2 Autoionization . . . . . . . . . .
32
2.5 Control and Non-linear Effects in Multiphoton Single Ionization
37
2.5.1 Control of Single Ionization Channels by Means of VUV
Pulses . . . . . . . . . . . . . . . . . . . . . . . . . . .
37
2.5.2 Non-linear Effects in (1 + 1)-REMPI . . . . . . . . . . .
39
2.5.3 Probing Nuclear Wave Packets in Molecular Excited
States . . . . . . . . . . . . . . . . . . . . . . . . . . . .
43
2.6 Future Perspectives . . . . . . . . . . . . . . . . . . . . . . . .
45
References . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .
46
ix
