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119. Aeschlimann M, Brixner T, Fischer A, Kramer C, Melchior P, Pfeiffer W, Schneider C, Struber C, Tuchscherer P, Voronine DV (2011) Coherent two-dimensional nanoscopy. Science
333(6050):1723–1726. https ://doi.org/10.1126/scien ce.12092 06
120. Liebel M, Toninelli C, van Hulst NF (2018) Room-temperature ultrafast nonlinear spectroscopy of
a single molecule. Nat Photonics 12(1):45–49. https ://doi.org/10.1038/s4156 6-017-0056-5
121. Mukamel S, Healion D, Zhang Y, Biggs JD (2013) Multidimensional attosecond resonant X-ray
spectroscopy of molecules: lessons from the optical regime. Annu Rev Phys Chem 64(1):101–127.
https ://doi.org/10.1146/annur ev-physc hem-04041 2-11002 1
122. Biggs JD, Zhang Y, Healion D, Mukamel S (2013) Multidimensional X-ray spectroscopy of valence
and core excitations in cysteine. J Chem Phys 138(14):144303. https ://doi.org/10.1063/1.47992 66
123. Kochise B, Yu Z, Markus K, Weijie H, Shaul M (2016) Multidimensional resonant nonlinear spectroscopy with coherent broadband X-ray pulses. Phys Scr T169:014002
124. Diels JC, Rudolph W (2006) Ultrashort laser pulse phenomena: fundamentals, techniques, and
applications on a femtosecond time scale. Optics and photonics, 2nd edn. Elsevier/Academic Press,
Amsterdam; Boston
125. Schmuttenmaer CA (2004) Exploring dynamics in the far-infrared with terahertz spectroscopy.
Chem Rev 104(4):1759–1779
126. Kampfrath T, Tanaka K, Nelson KA (2013) Resonant and nonresonant control over matter and
light by intense terahertz transients. Nat Photonics 7(9):680–690
127. Cho MH (2008) Coherent two-dimensional optical spectroscopy. Chem Rev 108(4):1331–1418.
https ://doi.org/10.1021/cr078 377b
128. Cho MH (2002) Ultrafast vibrational spectroscopy in condensed phases. PhysChemComm 5:40–
58. https ://doi.org/10.1039/b1108 98k
129. Dietze DR, Mathies RA (2016) Femtosecond stimulated Raman spectroscopy. ChemPhysChem
17(9):1224–1251
130. Kubarych KJ, Milne CJ, Miller RJD (2003) Fifth-order two-dimensional Raman spectroscopy: a
new direct probe of the liquid state. Int Rev Phys Chem 22(3):497–532
131. Rodriguez Y, Frei F, Cannizzo A, Feurer T (2015) Pulse-shaping assisted multidimensional coherent electronic spectroscopy. J Chem Phys 142(21):212451
132. Voronine DV, Abramavicius D, Mukamel S (2011) Coherent control protocol for separating
energy-transfer pathways in photosynthetic complexes by chiral multidimensional signals. J Phys
Chem A 115(18):4624–4629
133. Fuller FD, Ogilvie JP (2015) Experimental implementations of two-dimensional Fourier transform
electronic spectroscopy. Annu Rev Phys Chem 66(66):667–690
134. Bakulin AA, Morgan SE, Kehoe TB, Wilson MWB, Chin AW, Zigmantas D, Egorova D, Rao A
(2016) Nat Chem 8:16–23. https ://doi.org/10.1038/nchem .2371
135. Sarovar M, Ishizaki A, Fleming GR, Whaley KB (2010) Nat Phys 6:462–467. https ://doi.
org/10.1038/nphys 1652
136. Yan C, Nishida J, Yuan R et al (2016) J Am Chem Soc 138(30):9694–9703. https ://doi.
org/10.1021/jacs.6b055 89
137. Maj M, Lomont JP, Rich KL, Alperstein AM, Zanni MT (2018) Chem Sci 9:463. https ://doi.
org/10.1039/c7sc0 3789a
138. Lu J, Zhang Y, Hwang HY, Ofori-Okai BK, Fleischer S, Nelson KA (2016) PNAS
113(42):11800–11805
139. Mehlenbacher RD, McDonough TJ, Grechko M et al (2015) Nat Commun. https ://doi.org/10.1038/
ncomm s7732
140. Guo Z, Molesky BM, Cheshire TP, Moran AM (2015) J Chem Phys 143:124202
141. Roeding S, Klimovich N, Brixner T (2017) J Chem Phys 146:084201. https ://doi.
org/10.1063/1.49763 09
24
Reprinted from the journal
1 3
119. Aeschlimann M, Brixner T, Fischer A, Kramer C, Melchior P, Pfeiffer W, Schneider C, Struber C, Tuchscherer P, Voronine DV (2011) Coherent two-dimensional nanoscopy. Science
333(6050):1723–1726. https ://doi.org/10.1126/scien ce.12092 06
120. Liebel M, Toninelli C, van Hulst NF (2018) Room-temperature ultrafast nonlinear spectroscopy of
a single molecule. Nat Photonics 12(1):45–49. https ://doi.org/10.1038/s4156 6-017-0056-5
121. Mukamel S, Healion D, Zhang Y, Biggs JD (2013) Multidimensional attosecond resonant X-ray
spectroscopy of molecules: lessons from the optical regime. Annu Rev Phys Chem 64(1):101–127.
https ://doi.org/10.1146/annur ev-physc hem-04041 2-11002 1
122. Biggs JD, Zhang Y, Healion D, Mukamel S (2013) Multidimensional X-ray spectroscopy of valence
and core excitations in cysteine. J Chem Phys 138(14):144303. https ://doi.org/10.1063/1.47992 66
123. Kochise B, Yu Z, Markus K, Weijie H, Shaul M (2016) Multidimensional resonant nonlinear spectroscopy with coherent broadband X-ray pulses. Phys Scr T169:014002
124. Diels JC, Rudolph W (2006) Ultrashort laser pulse phenomena: fundamentals, techniques, and
applications on a femtosecond time scale. Optics and photonics, 2nd edn. Elsevier/Academic Press,
Amsterdam; Boston
125. Schmuttenmaer CA (2004) Exploring dynamics in the far-infrared with terahertz spectroscopy.
Chem Rev 104(4):1759–1779
126. Kampfrath T, Tanaka K, Nelson KA (2013) Resonant and nonresonant control over matter and
light by intense terahertz transients. Nat Photonics 7(9):680–690
127. Cho MH (2008) Coherent two-dimensional optical spectroscopy. Chem Rev 108(4):1331–1418.
https ://doi.org/10.1021/cr078 377b
128. Cho MH (2002) Ultrafast vibrational spectroscopy in condensed phases. PhysChemComm 5:40–
58. https ://doi.org/10.1039/b1108 98k
129. Dietze DR, Mathies RA (2016) Femtosecond stimulated Raman spectroscopy. ChemPhysChem
17(9):1224–1251
130. Kubarych KJ, Milne CJ, Miller RJD (2003) Fifth-order two-dimensional Raman spectroscopy: a
new direct probe of the liquid state. Int Rev Phys Chem 22(3):497–532
131. Rodriguez Y, Frei F, Cannizzo A, Feurer T (2015) Pulse-shaping assisted multidimensional coherent electronic spectroscopy. J Chem Phys 142(21):212451
132. Voronine DV, Abramavicius D, Mukamel S (2011) Coherent control protocol for separating
energy-transfer pathways in photosynthetic complexes by chiral multidimensional signals. J Phys
Chem A 115(18):4624–4629
133. Fuller FD, Ogilvie JP (2015) Experimental implementations of two-dimensional Fourier transform
electronic spectroscopy. Annu Rev Phys Chem 66(66):667–690
134. Bakulin AA, Morgan SE, Kehoe TB, Wilson MWB, Chin AW, Zigmantas D, Egorova D, Rao A
(2016) Nat Chem 8:16–23. https ://doi.org/10.1038/nchem .2371
135. Sarovar M, Ishizaki A, Fleming GR, Whaley KB (2010) Nat Phys 6:462–467. https ://doi.
org/10.1038/nphys 1652
136. Yan C, Nishida J, Yuan R et al (2016) J Am Chem Soc 138(30):9694–9703. https ://doi.
org/10.1021/jacs.6b055 89
137. Maj M, Lomont JP, Rich KL, Alperstein AM, Zanni MT (2018) Chem Sci 9:463. https ://doi.
org/10.1039/c7sc0 3789a
138. Lu J, Zhang Y, Hwang HY, Ofori-Okai BK, Fleischer S, Nelson KA (2016) PNAS
113(42):11800–11805
139. Mehlenbacher RD, McDonough TJ, Grechko M et al (2015) Nat Commun. https ://doi.org/10.1038/
ncomm s7732
140. Guo Z, Molesky BM, Cheshire TP, Moran AM (2015) J Chem Phys 143:124202
141. Roeding S, Klimovich N, Brixner T (2017) J Chem Phys 146:084201. https ://doi.
org/10.1063/1.49763 09
24
Reprinted from the journal