189. Nihonyanagi S, Mondal JA, Yamaguchi S, Tahara T (2013) Structure and dynamics of interfacial
water studied by heterodyne-detected vibrational sum-frequency generation. Annu Rev Phys Chem
64:579–603. doi:10.1146/annurev-physchem-040412-110138
190. Shen YR, Ostroverkhov V (2006) Sum-frequency vibrational spectroscopy on water interfaces:
polar orientation of water molecules at interfaces. Chem Rev 106:1140–1154. doi:10.1021/
cr040377d
191. Ishiyama T, Imamura T, Morita A (2014) Theoretical studies of structures and vibrational sum
frequency generation spectra at aqueous interfaces. Chem Rev 114:8447–8470
192. Laaser JE, Zanni MT (2013) Extracting structural information from the polarization dependence of
one- and two-dimensional sum frequency generation spectra. J Phys Chem A 117:5875–5890
193. Ho J-J, Skoff DR, Ghosh A, Zanni MT (2015) Structural characterization of single-stranded DNA
monolayers using two-dimensional sum frequency generation spectroscopy. J Phys Chem B
119:10586–10596. doi:10.1021/acs.jpcb.5b07078
194. Laaser JE, Skoff DR, Ho J et al (2014) Two-dimensional sum-frequency generation reveals
structure and dynamics of a surface-bound peptide. J Am Chem Soc 136:956–962
195. Zhang Z, Piatkowski L, Bakker HJ, Bonn M (2011) Communication: interfacial water structure
revealed by ultrafast two-dimensional surface vibrational spectroscopy. J Chem Phys 135:18–21.
doi:10.1063/1.3605657
196. Hsieh C-S, Okuno M, Hunger J et al (2014) Aqueous heterogeneity at the air/water interface
revealed by 2D-HD-SFG spectroscopy. Angew Chem Int Ed Engl 53:8146–8149. doi:10.1002/anie.
201402566
197. Nagata Y, Mukamel S (2011) Spectral diffusion at the water/lipid interface revealed by twodimensional fourth-order optical spectroscopy: a classical simulation study. J Am Chem Soc
133:3276–3279. doi:10.1021/ja110748s
198. Singh PC, Inoue KI, Nihonyanagi S et al (2016) Femtosecond hydrogen bond dynamics of bulk-like
and bound water at positively and negatively charged lipid interfaces revealed by 2D HD-VSFG
spectroscopy. Angew Chemie Int Ed 55:10621–10625. doi:10.1002/anie.201603676
199. Livingstone RA, Nagata Y, Bonn M, Backus EHG (2015) Two types of water at the watersurfactant interface revealed by time-resolved vibrational spectroscopy. J Am Chem Soc
137:14912–14919. doi:10.1021/jacs.5b07845
200. Singh PC, Nihonyanagi S, Yamaguchi S, Tahara T (2012) Ultrafast vibrational dynamics of water at
a charged interface revealed by two-dimensional heterodyne-detected vibrational sum frequency
generation. J Chem Phys 137(094706):1–6. doi:10.1063/1.4747828
201. Inoue KI, Nihonyanagi S, Singh PC et al (2015) 2D heterodyne-detected sum frequency generation
study on the ultrafast vibrational dynamics of H2O and HOD water at charged interfaces. J Chem
Phys 142(212431):1–12. doi:10.1063/1.4918644
202. Piatkowski L, Zhang Z, Backus EHG et al (2014) Extreme surface propensity of halide ions in
water. Nat Commun 5:4083. doi:10.1038/ncomms5083
203. Fecko CJ, Eaves JD, Loparo JJ et al (2003) Ultrafast hydrogen-bond dynamics in the infrared.
Science 301:1698–1702
204. Kraack JP, Lotti D, Hamm P (2014) Ultrafast, multidimensional attenuated total reflectance
spectroscopy of adsorbates at metal surfaces. J Phys Chem Lett 5:2325–2329
205. Kraack JP, Kaech A, Hamm P (2017) Molecule-specific interactions of diatomic adsorbates at
metal-liquid interfaces. Struct Dyn 4(044009):1–14. doi:10.1063/1.4978894
206. Zamadar M, Asaoka S, Grills DC, Miller JR (2013) Giant infrared absorption bands of electrons and
holes in conjugated molecules. Nat Commun 4:2818. doi:10.1038/ncomms3818
207. Bertie JE, Lan Z (1996) Infrared intensities of liquids XX: the intensity of the OH stretching band of
liquid water revisited, and the best current values of the optical constants of H2O(l) at 25 C between
15,000 and 1 cm
-1 . Appl Spectrosc 50:1047–1057. doi:10.1366/0003702963905385
208. Yan C, Nishida J, Yuan R, Fayer MD (2016) Water of hydration dynamics in minerals gypsum and
bassanite: ultrafast 2D IR spectroscopy of rocks. J Am Chem Soc 138:9694–9703. doi:10.1021/jacs.
6b05589
209. Bakulin AA, Cringus D, Pieniazek PA et al (2013) Dynamics of water confined in reversed
micelles: multidimensional vibrational spectroscopy study. J Phys Chem B 117:15545–15558.
doi:10.1021/jp405853j
210. Bagchi B (2005) Water dynamics in the hydration layer around proteins and micelles. Chem Rev
105:3197–3219. doi:10.1021/cr020661?
Top Curr Chem (Z) (2017) 375:86
123
197
Reprinted from the journal
water studied by heterodyne-detected vibrational sum-frequency generation. Annu Rev Phys Chem
64:579–603. doi:10.1146/annurev-physchem-040412-110138
190. Shen YR, Ostroverkhov V (2006) Sum-frequency vibrational spectroscopy on water interfaces:
polar orientation of water molecules at interfaces. Chem Rev 106:1140–1154. doi:10.1021/
cr040377d
191. Ishiyama T, Imamura T, Morita A (2014) Theoretical studies of structures and vibrational sum
frequency generation spectra at aqueous interfaces. Chem Rev 114:8447–8470
192. Laaser JE, Zanni MT (2013) Extracting structural information from the polarization dependence of
one- and two-dimensional sum frequency generation spectra. J Phys Chem A 117:5875–5890
193. Ho J-J, Skoff DR, Ghosh A, Zanni MT (2015) Structural characterization of single-stranded DNA
monolayers using two-dimensional sum frequency generation spectroscopy. J Phys Chem B
119:10586–10596. doi:10.1021/acs.jpcb.5b07078
194. Laaser JE, Skoff DR, Ho J et al (2014) Two-dimensional sum-frequency generation reveals
structure and dynamics of a surface-bound peptide. J Am Chem Soc 136:956–962
195. Zhang Z, Piatkowski L, Bakker HJ, Bonn M (2011) Communication: interfacial water structure
revealed by ultrafast two-dimensional surface vibrational spectroscopy. J Chem Phys 135:18–21.
doi:10.1063/1.3605657
196. Hsieh C-S, Okuno M, Hunger J et al (2014) Aqueous heterogeneity at the air/water interface
revealed by 2D-HD-SFG spectroscopy. Angew Chem Int Ed Engl 53:8146–8149. doi:10.1002/anie.
201402566
197. Nagata Y, Mukamel S (2011) Spectral diffusion at the water/lipid interface revealed by twodimensional fourth-order optical spectroscopy: a classical simulation study. J Am Chem Soc
133:3276–3279. doi:10.1021/ja110748s
198. Singh PC, Inoue KI, Nihonyanagi S et al (2016) Femtosecond hydrogen bond dynamics of bulk-like
and bound water at positively and negatively charged lipid interfaces revealed by 2D HD-VSFG
spectroscopy. Angew Chemie Int Ed 55:10621–10625. doi:10.1002/anie.201603676
199. Livingstone RA, Nagata Y, Bonn M, Backus EHG (2015) Two types of water at the watersurfactant interface revealed by time-resolved vibrational spectroscopy. J Am Chem Soc
137:14912–14919. doi:10.1021/jacs.5b07845
200. Singh PC, Nihonyanagi S, Yamaguchi S, Tahara T (2012) Ultrafast vibrational dynamics of water at
a charged interface revealed by two-dimensional heterodyne-detected vibrational sum frequency
generation. J Chem Phys 137(094706):1–6. doi:10.1063/1.4747828
201. Inoue KI, Nihonyanagi S, Singh PC et al (2015) 2D heterodyne-detected sum frequency generation
study on the ultrafast vibrational dynamics of H2O and HOD water at charged interfaces. J Chem
Phys 142(212431):1–12. doi:10.1063/1.4918644
202. Piatkowski L, Zhang Z, Backus EHG et al (2014) Extreme surface propensity of halide ions in
water. Nat Commun 5:4083. doi:10.1038/ncomms5083
203. Fecko CJ, Eaves JD, Loparo JJ et al (2003) Ultrafast hydrogen-bond dynamics in the infrared.
Science 301:1698–1702
204. Kraack JP, Lotti D, Hamm P (2014) Ultrafast, multidimensional attenuated total reflectance
spectroscopy of adsorbates at metal surfaces. J Phys Chem Lett 5:2325–2329
205. Kraack JP, Kaech A, Hamm P (2017) Molecule-specific interactions of diatomic adsorbates at
metal-liquid interfaces. Struct Dyn 4(044009):1–14. doi:10.1063/1.4978894
206. Zamadar M, Asaoka S, Grills DC, Miller JR (2013) Giant infrared absorption bands of electrons and
holes in conjugated molecules. Nat Commun 4:2818. doi:10.1038/ncomms3818
207. Bertie JE, Lan Z (1996) Infrared intensities of liquids XX: the intensity of the OH stretching band of
liquid water revisited, and the best current values of the optical constants of H2O(l) at 25 C between
15,000 and 1 cm
-1 . Appl Spectrosc 50:1047–1057. doi:10.1366/0003702963905385
208. Yan C, Nishida J, Yuan R, Fayer MD (2016) Water of hydration dynamics in minerals gypsum and
bassanite: ultrafast 2D IR spectroscopy of rocks. J Am Chem Soc 138:9694–9703. doi:10.1021/jacs.
6b05589
209. Bakulin AA, Cringus D, Pieniazek PA et al (2013) Dynamics of water confined in reversed
micelles: multidimensional vibrational spectroscopy study. J Phys Chem B 117:15545–15558.
doi:10.1021/jp405853j
210. Bagchi B (2005) Water dynamics in the hydration layer around proteins and micelles. Chem Rev
105:3197–3219. doi:10.1021/cr020661?
Top Curr Chem (Z) (2017) 375:86
123
197
Reprinted from the journal